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Methane steroids steroids, CO, methyl formate, acetaldehyde and hydrogen were detected in the reactor and the concentrations of all but CO, were greatly increased for TiO2:Rh LHCII compared to TiO2:Rh in visible light experiments.Ordinary differential equation (ODE) models were developed for CO2 photoreduction to investigate the steady state concentrations of the products and make predictions about their response to different experimental parameters. The light absorption was confirmed as a viable optimisation target for increasing product concentrations. A stochastic discrete spatial model was also developed which showed that spatial effects are important for reduction rates and that the hydrophilicity of the catalyst may lead to reaction stalling.It was concluded that, if issues with LHCII stability and maximising light absorption without interfering with catalysis are dealt with, LHCII could be a promising method for enhancing CO2 photoreduction with the appropriate catalyst..

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